Download Oxide Materials at the Two-Dimensional Limit by Falko P. Netzer, Alessandro Fortunelli PDF

By Falko P. Netzer, Alessandro Fortunelli

This ebook summarizes the present wisdom of two-dimensional oxide fabrics. the basic homes of 2-D oxide platforms are explored by way of atomic constitution, digital habit and floor chemistry. the idea that of polarity in picking the steadiness of 2-D oxide layers is tested, cost move results in ultrathin oxide movies are reviewed in addition to the position of defects in 2-D oxide motion pictures. the unconventional constitution options that practice in oxide structures of low dimensionality are addressed, and a bankruptcy giving an outline of cutting-edge theoretical equipment for digital constitution choice of nanostructured oxides is integrated. detailed emphasis is given to a balanced view from the experimental and the theoretical aspect. Two-dimensional fabrics, and 2-D oxides particularly, have awesome habit as a result of dimensionality and proximity results. numerous chapters deal with prototypical version structures as illustrative examples to debate the atypical actual and chemical houses of 2-D oxide platforms. The chapters are written via well known specialists within the field.

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Extra resources for Oxide Materials at the Two-Dimensional Limit

Example text

Adapted from [81, 82] not particular to the Cu-tungstate phase, but appears to be of a more general validity. For example, Ni-tungstate NiWO4 on Ni(110) has been fabricated by chemical reaction of NiO/Ni(110) with (WO3)3 clusters [86], and a surface Fe-tungstate phase has been generated by the interfacial reaction of the FeO(111) bilayer phase on Pt(111) (see Sect. 2) with (WO3)3 clusters [87]. The first step in the latter interface reaction between FeO(111)/Pt(111) and (WO3)3 clusters has been observed by Li et al.

Adapted from [94] different phases, since subtle variations in the thermodynamic parameters, often below the control of the experimenter, may drive the system into a different structure. It is therefore a challenge in these systems with multi-structure phase diagrams to reproducibly prepare a particular phase, which sometimes even cannot be prepared as a single phase at the surface. This is detrimental for the structure characterization, since a combination of several experimental techniques is often necessary, including area averaging techniques besides the space-resolved STM, to unravel a complex oxide structure.

9a, left panel. The (2 × 1) structure is polar and its total energy as calculated by DFT is only at a local minimum: it is thus a meta-stable phase, with Fig. 0 V of the (2 × 1) phase of MnO on Ag(100) (blue Mn atoms; red O atoms). 5 eV) or B3PW91 (in parenthesis). P. Netzer and S. Surnev the MnO(100)1 × 1 phase being the thermodynamically stable ground state. The (2 × 1) phase, which in the case of MnO/Ag(100) is the predominant phase observed experimentally for the monolayer, must therefore be kinetically stabilized during growth.

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